the Bronco and the Disco/RRC have very similar bushings at the frame stock. as you lift these trucks you preload the stock bushings and limit down travel or droop. We were doing heim jointed front radius arms on the bronco's 30 years ago to prevent this binding. Add in a cut and rotate of the inner 'C' to correct caster and you were good to go. There were lots of bronco's running 38-44" tires in the group I started wheeling with 30 years ago.
the bronco's front suspension is far from obsolete, infact it was well ahead of its time . The hot set up used to be to graft on the radius arms from the front onto the rear and get rid of the leaf springs alltogether. this would yeild a very compliant suspension that would flex like no tomorow.
With the Disco/RRC instead of going to a heim jointed front radius arm the most common change is to offset the frame end of the radius arm so the radius arm goes through the bushing center line and does not preload the bushing. This is a good fix in that you still have the rubber bushing to isolate the noise from the passenger compartment. allthough the heim joints or urathane core johnny joints are not at all limited in flex as the stock bushings are, the noise transmission from them may be more then desired by a overland traveller might want to deal with.
there is one other important modification needed once you reach 3" or more of lift with a Disco/RRC. once you rotate the swivel balls the front drag link location changes as well. this change moves the panhard bar and drag link out of a parralel position. this causes the steering to see-saw over bumps. to do away with this you will need to raise the location of the Panhard bar on the axle housing so that the two are once again in the same plane. this then makes the truck drive like it should.
As I stated before you need to look at the front suspension and steering as a whole and address all the issues. once you do that driving quality returns to that of a stock Land Rover and you will feel the extra steps are worth it.
From your description it sounds like the Discovery's front suspension is very similar to the early Bronco's- what I suspected, but since I've never seen one, I wasn't sure. The issues you describe are the same ones I've been through with my Bronco as I've evolved the suspension over the 13 years I've owned it.
Longer springs lifted it (currently 4 inches). I cut the inner knuckles off the Dana 44 axle housing and rotated them back 10 degrees to get the caster back while keeping the correct pinion angle.
The addition of a longer drivetrain (NV4500 & Atlas II) moved the front yoke on the transfer case 6 inches aft. This gave me some front driveshaft vibration since the pinion no longer stayed aligned (pointed at the t-case yoke) as the suspension cycled. 6 inch longer radius arms with Currie Johnie joints took care of that- also gave me another degree of caster.
Meanwhile, rotating the knuckles on the axles rotated the tie rod up & aft, along with the drag link. Since I had already moved the tie rod & drag link above the knuckles, it really threw the drag link/ panhard rod relationship out of whack. I fabricated a new panhard mount on the axle that is outboard of the radius arm rather than inboard. The drag link and panhard rod are once again parallel, and the outboard upper mount means that the two rods are now the same length. So they remain parallel as the suspension moves.
There are probably more details, but I don't remember them offhand. In the end, I've got about 6 degrees of positive caster and very stable steering that readily returns to center, with no bumpsteer.
Whew! Now I need to find a Discovery to crawl under so I can see it for myself.