I've had 2 converted bifuel vehicles, both newer 1/2 ton trucks, one for business, one personal.
Overall, I loved it. IMO, the only major downside is fuel availability. CNG can be very hard to come by in certain areas of the country. Sticking with bifuel solves that, but it always feels wrong to be running on gasoline in a vehicle you've spend thousands converting to run on CNG.
On an older vehicle like yours, the installation is greatly simplified. Once you get into sequential port injection CNG systems, the tuning gets complicated and I found both my vehicles visiting my CNG tuner pretty often until all the little issues were sorted out. Often times the vehicle was working perfectly, but would throw a Check Engine light due to operating out of emissions specs (ECU would assume it was running too lean).
Tank size versus range can be a difficult decision. I had a 24.5 gallon equivalent CNG tank in my personal truck and that was just too big. I gave up more cargo space than I would have liked. In most full-size trucks, a 21 gallon tank is the way to go as it's width allows it to sit down lower in the truck bed, even allowing for a tonneau cover.
In a Suburban, you're either going to give up most of your cargo room to CNG tanks to get any significant range or you're going to mount 10 gallons of CNG in place of your spare, which cut's ground clearance and gives you an annoyingly short range. I highly recommend the first option, 18-21 gallons of fuel allows you a normal range, you'll quickly tire of filling up every 1-2 days with a 10 gallon tank.